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Cryogenic Exfoliation of Non-layered Magnesium into Two-Dimensional Crystals
Zhang, Chen; Xu, Yingfeng; Lu, Ping; Wei, Chenyang; Zhu, Chenxi; Yao, Heliang; Xu, Fangfang; Shi, Jianlin
2019-06-24
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN1433-7851
Volume58Issue:26Pages:8814
SubtypeArticle
AbstractPhysical exfoliation of layered precursors is one of the most prevailing techniques to prepare two-dimensional (2D) crystals, which, however, is considered to be intrinsically inapplicable to non-layered bulks. Now, plane cleavage differentiation is identified in metallic magnesium at cryogenic temperature (CT), and a cryogenic exfoliation strategy of non-layered magnesium into 2D crystals is developed. The cleavage anisotropy of the Mg lattice in response to the external mechanical stress originates from the CT-induced specific inactivation of basal slip, which results in the basal cleavage perpendicular to c axis. The exfoliated novel 2D Mg crystals exhibit remarkable localized surface plasmon resonances, holding great promise for the applications in harvesting and converting solar energy. Beyond creating a new member for the burgeoning 2D family, this study may provide a useful tool for the physical exfoliations of various non-layered materials.
Keywordcryogenic cleavage metallic crystals physical exfoliation two-dimensional Mg
DOI10.1002/anie.201903485
Language英语
WOS Research AreaChemistry
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://ir.sic.ac.cn/handle/331005/27039
Collection中国科学院上海硅酸盐研究所
Recommended Citation
GB/T 7714
Zhang, Chen,Xu, Yingfeng,Lu, Ping,et al. Cryogenic Exfoliation of Non-layered Magnesium into Two-Dimensional Crystals[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(26):8814.
APA Zhang, Chen.,Xu, Yingfeng.,Lu, Ping.,Wei, Chenyang.,Zhu, Chenxi.,...&Shi, Jianlin.(2019).Cryogenic Exfoliation of Non-layered Magnesium into Two-Dimensional Crystals.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(26),8814.
MLA Zhang, Chen,et al."Cryogenic Exfoliation of Non-layered Magnesium into Two-Dimensional Crystals".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.26(2019):8814.
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