SIC OpenIR
Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell
Li, Shuangbin1,2; Pan, Wenzhi1; Wang, Shaorong3; Meng, Xie1; Jiang, Cairong2; Irvine, John T.S.2
2017
发表期刊International Journal of Hydrogen Energy
ISSN03603199
卷号42期号:25页码:16279-16287
摘要In this work, three processed carbon fuels including activated carbon, carbon black and graphite have been employed to investigate influence of the chemical and physical properties of carbon on the HDCFC performance in different anode atmospheres at 650–800 °C. The results reveal that the electrochemical activity is strongly dependent on crystalline structure, thermal stability and textural properties of carbon fuels. The activated carbon samples demonstrate a better performance with a peak power density of 326 mW cm−2in CO2at 750 °C, compared to 147 and 59 mW cm−2with carbon black and graphite samples, respectively. Compared to the ohmic resistance, the polarization resistance plays a more dominated role in the cell performance. When replacing N2by CO2purge gas, the power density is the strongly temperature dependent due to the Boudouard reaction. © 2017 Hydrogen Energy Publications LLC
DOI10.1016/j.ijhydene.2017.05.150
EI入藏号20172403766654
EI主题词Direct carbon fuel cells (DCFC)
EI分类号702.2 Fuel Cells - 803 Chemical Agents and Basic Industrial Chemicals - 804 Chemical Products Generally - 804.2 Inorganic Compounds - 931.2 Physical Properties of Gases, Liquids and Solids
引用统计
文献类型期刊论文
条目标识符http://ir.sic.ac.cn/handle/331005/25644
专题中国科学院上海硅酸盐研究所
作者单位1.CAS Key Laboratory of Materials for Energy Conversion, Shanghai Institute of Ceramics, Chinese Academy of Sciences (SICCAS), China;
2.School of Chemistry, University of St Andrews, KY16 9ST, United Kingdom;
3.School of Chemical Engineering & Technology, China University of Mining and Technology, China
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GB/T 7714
Li, Shuangbin,Pan, Wenzhi,Wang, Shaorong,et al. Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell[J]. International Journal of Hydrogen Energy,2017,42(25):16279-16287.
APA Li, Shuangbin,Pan, Wenzhi,Wang, Shaorong,Meng, Xie,Jiang, Cairong,&Irvine, John T.S..(2017).Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell.International Journal of Hydrogen Energy,42(25),16279-16287.
MLA Li, Shuangbin,et al."Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell".International Journal of Hydrogen Energy 42.25(2017):16279-16287.
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