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Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell
Li, Shuangbin1,2; Pan, Wenzhi1; Wang, Shaorong3; Meng, Xie1; Jiang, Cairong2; Irvine, John T.S.2
2017
Source PublicationInternational Journal of Hydrogen Energy
ISSN03603199
Volume42Issue:25Pages:16279-16287
AbstractIn this work, three processed carbon fuels including activated carbon, carbon black and graphite have been employed to investigate influence of the chemical and physical properties of carbon on the HDCFC performance in different anode atmospheres at 650–800 °C. The results reveal that the electrochemical activity is strongly dependent on crystalline structure, thermal stability and textural properties of carbon fuels. The activated carbon samples demonstrate a better performance with a peak power density of 326 mW cm−2in CO2at 750 °C, compared to 147 and 59 mW cm−2with carbon black and graphite samples, respectively. Compared to the ohmic resistance, the polarization resistance plays a more dominated role in the cell performance. When replacing N2by CO2purge gas, the power density is the strongly temperature dependent due to the Boudouard reaction. © 2017 Hydrogen Energy Publications LLC
DOI10.1016/j.ijhydene.2017.05.150
EI Accession Number20172403766654
EI KeywordsDirect carbon fuel cells (DCFC)
EI Classification Number702.2 Fuel Cells - 803 Chemical Agents and Basic Industrial Chemicals - 804 Chemical Products Generally - 804.2 Inorganic Compounds - 931.2 Physical Properties of Gases, Liquids and Solids
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Document Type期刊论文
Identifierhttp://ir.sic.ac.cn/handle/331005/25644
Collection中国科学院上海硅酸盐研究所
Affiliation1.CAS Key Laboratory of Materials for Energy Conversion, Shanghai Institute of Ceramics, Chinese Academy of Sciences (SICCAS), China;
2.School of Chemistry, University of St Andrews, KY16 9ST, United Kingdom;
3.School of Chemical Engineering & Technology, China University of Mining and Technology, China
Recommended Citation
GB/T 7714
Li, Shuangbin,Pan, Wenzhi,Wang, Shaorong,et al. Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell[J]. International Journal of Hydrogen Energy,2017,42(25):16279-16287.
APA Li, Shuangbin,Pan, Wenzhi,Wang, Shaorong,Meng, Xie,Jiang, Cairong,&Irvine, John T.S..(2017).Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell.International Journal of Hydrogen Energy,42(25),16279-16287.
MLA Li, Shuangbin,et al."Electrochemical performance of different carbon fuels on a hybrid direct carbon fuel cell".International Journal of Hydrogen Energy 42.25(2017):16279-16287.
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